Self-assembly of oligomeric structures on gold

COLL 424

Bo Liedberg, Divisions of Sensor Science and Molecular Physics, Divisions of Sensor Science and Molecular Physics, Linköping University, Department of Physics and Measurement Technology, Linkoping, S-58183, Sweden
This contribution describes the self-assembly of alkane thiols and disulphides bearing complex tail groups including, e.g. oligo(ethylene glycols), oligosaccharides and polypeptides. A few examples are given where so-called conformational gradients based on oligo(ethylene glycols) are used to study the protein rejecting properties of non-natural surfaces. The same type of gradients is also used to fine tune and optimise the immobilisation and binding characteristics of sensing surfaces relying the biotin/streptavidin platform. A broad spectrum of oligosaccharide terminated thiols and disuphides recently have been synthesized at our laboratory for applications in biosensing and molecular recognition. Oligosaccharide surfaces bearing b-D-Gal-(1→3)-D-GalNAc tails are also used in a biomimetic materials science project aiming at mimicking the properties of anti-freeze glyco proteins (AFGP). Finally I describe a new class of helix-loop-helix polypeptides that can be used as a scaffold for site-selective attachment of, in principle, any type of ligand. A few examples describing their applications in the evergrowing fields of proteomics and receptor mimicking are highlighted
 

Adamson Award Symposium Honoring Dave Allara and Ralph Nuzzo

Division of Colloid and Surface Chemistry
The 225th ACS National Meeting, New Orleans, LA, March 23-27, 2003